Effect of confinement on ammonia inversion

dc.contributor.authorSathyamurthy, Narayanasami
dc.date.accessioned2023-08-21T08:24:05Z
dc.date.available2023-08-21T08:24:05Z
dc.date.issued2021
dc.descriptionOnly IISERM authors are available in the record.en_US
dc.description.abstractThe effect of confinement on ammonia inversion inside C50 (D5h) and C60 (Ih) fullerenes has been investigated. Calculations at the DFT(M06-2X)/6-311G** level of theory suggest that NH3 is stable inside both C50 and C60 by −8.6 and −23.8 kcal mol−1, respectively. While the barrier for inversion of the free NH3 molecule is estimated to be 1896 cm−1, it increases to 1972 cm−1 and 2108 cm−1, respectively, inside C50 and C60. The results also reveal that the magnitude of splitting of the bound states below the barrier in the symmetric double-well potential decreases inside both the C50 and C60 cages.en_US
dc.identifier.citationThe European Physical Journal D, 75(3).en_US
dc.identifier.urihttps://doi.org/10.1140/epjd/s10053-021-00118-3
dc.identifier.urihttp://hdl.handle.net/123456789/4939
dc.language.isoen_USen_US
dc.publisherSpringer Linken_US
dc.subjectconfinementen_US
dc.subjectammoniaen_US
dc.subjectEffecten_US
dc.subjectinversionen_US
dc.titleEffect of confinement on ammonia inversionen_US
dc.typeArticleen_US

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