Interpretation of the accidental predissociation of the E1Π state of CO

dc.contributor.authorSathyamurthy, N.
dc.date.accessioned2020-12-10T07:50:03Z
dc.date.available2020-12-10T07:50:03Z
dc.date.issued2014
dc.descriptionOnly IISERM authors are available in the record.
dc.description.abstractA special case of predissociation, known as indirect or accidental predissociation observed in the Rydberg E1Π bound state of CO is discussed. We resort to ab initio potentials in order to determine the plausible mechanism for this predissociation. Values of the predissociation width for the valence k3Π state of CO, as obtained from Fermi's golden rule, are also reported. The predissociation width obtained for the mixed E 1Π (v = 1, J = 7) state is 0.033 cm-1 compared to the experimental value of 0.034 cm-1. The mixed E - E′ state with J = 28, v = 0 is found to be in near resonance condition with the k3Π (v = 4, J = 28) state, thus providing the means to indirect predissociation.en_US
dc.identifier.citationJournal of Chemical Physics,140(16)en_US
dc.identifier.otherhttps://doi.org/10.1063/1.4871109
dc.identifier.urihttps://aip.scitation.org/doi/10.1063/1.4871109
dc.identifier.urihttp://hdl.handle.net/123456789/2966
dc.language.isoenen_US
dc.publisherAmerican Institute of Physicsen_US
dc.subjectPre-dissociationen_US
dc.subjectRydbergen_US
dc.subjectBound stateen_US
dc.titleInterpretation of the accidental predissociation of the E1Π state of COen_US
dc.typeArticleen_US

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